GENERAL STUDY OF CLASSICAL AND NONCLASSICAL CONTRIBUTIONS OF TWO PHOTON ABSORPTION PROCESS IN ORGANIC MOLECULES

Freiman Estiven Triana Arango (2023, [Tesis de doctorado])

"Two-photon absorption (TPA), a nonlinear optical phenomenon, is gaining attention for applications like laser scanning, microscopy, and therapy. Recent research explores entangled two photon absorption (ETPA) using correlated photons but faces debates regarding its magnitude and detection. This study introduces a novel method using changes in Hong-Ou-Mandel (HOM) interferogram visibility to probe ETPA's presence. It employs Rhodamine B dye and entangled photons at around 800nm to investigate conditions conducive to observing ETPA-induced changes. This innovative approach distinguishes genuine ETPA signals from linear optical losses often masquerading as ETPA effects, addressing a significant field challenge."

Two-photon absorption Entangled two-photon absorption Hong-Ou-Mandel HOM dip visibility Joint Spectral Intensity Entangled photons CIENCIAS FÍSICO MATEMÁTICAS Y CIENCIAS DE LA TIERRA FÍSICA ÓPTICA OPTICA NO LINEAL OPTICA NO LINEAL